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Additional resources for Chemistry, emission control, radioactive pollution and indoor air quality
The application of CO2 capture in an IGCC will decrease the NOx emissions per MJprimary as relatively less gas is combusted in the gas turbine per unit of primary energy input. This outcome strongly depends on the assumption that the issue of NOx formation in a gas turbine fired with fuel gas with a high hydrogen content is solved by turbine manufacturers. The flame temperature is namely dependent on the gas composition and heating value. Both of these will change when applying CO2 capture. If dilution with steam or nitrogen is not applied, the flame temperature during firing of hydrogen rich fuel will increase resulting in an increase in NOx formation.
The application of precombustion CO2 capture in an IGCC is assumed to enhance the SO2 removal. The application of CO2 capture is likely to result in a decrease of the emission of SO2 per MJprimary, but depending on the efficiency penalty may result in an increase per kWh. Both increase and decrease per kWh have been reported in literature. The reduction per MJprimary is expected to be lower compared to the post-combustion and oxyfuel combustion technologies (see Fig. 2). With pre-combustion it is also possible to yield a stream of CO2 with H2S and co-inject this into the underground.
2007;Weisser 2007;Koornneef, van Keulen et al. 2008;Odeh and Cockerill 2008;RECCS 2008;Bauer and Heck 2009;Markewitz, Schreiber et al. 2009;NEEDS 2009;Nie 2009;Pehnt and Henkel 2009;Schreiber, Zapp et al. 2009;Korre, Nie et al. 2010) (Waku, Tamura et al. 1995;Akai, Nomura et al. 1997;Lombardi 2003;Tzimas, Mercier et al. 2007;Viebahn, Nitsch et al. 2007;Weisser 2007;Odeh and Cockerill 2008;RECCS 2008;Pehnt and Henkel 2009) (Viebahn, Nitsch et al. 2007;RECCS 2008;Bauer and Heck 2009;NEEDS 2009;Nie 2009;Pehnt and Henkel 2009) (Lombardi 2003;Spath and Mann 2004;Sundkvist, Klang et al.